Personal information

polymers, biobased materials, sustainability, battery membranes, drug delivery, plastics upcycling
United States

Biography

Thomas is the Allan & Myra Ferguson Distinguished Professor of Chemical & Biomolecular Engineering at the University of Delaware (UD) with a joint appointment in Materials Science & Engineering. He is Director of the Center for Research in Soft matter & Polymers (CRiSP), Director of the NSF MRSEC at UD called CHARM (Center for Hybrid, Active, and Responsive Materials) and Deputy Director of the DOE EFRC at UD called CPI (Center for Plastics Innovation). His research interests include nanostructured assemblies for targeted drug delivery and gene therapy, polymeric materials for bio-separation and ion-conduction membranes, nanostructured soft materials from biobased and plastics waste feedstocks, and polymer films for nanotemplating. He was elected a Fellow of the American Physical Society in 2017, Royal Society of Chemistry (FRSC) in 2018, American Institute for Medical and Biological Engineering in 2021, Polymers Division of the American Chemical Society in 2021, American Chemical Society in 2021, and the National Academy of Inventors in 2022, and Polymeric Materials Science and Engineering Division of the American Chemical Society in 2023. Thomas is also co-founder and Chief Scientific Officer of Lignolix, Inc. – a start-up focused on valorization of biomass waste. He has received several honors and awards including: the William W. Grimes Award (AIChE, 2021), Percy L. Julian Award (NOBCChE, 2020); John H. Dillon Medal (APS, 2016); Owens-Corning Early Career Award (AIChE, 2015), among others. Thomas is a member of the DOE Basic Energy Sciences Advisory Committee and a member of advisory boards/committees in the private and financial sector.

Activities

Employment (3)

Lignolix, Inc: Wilmington, DE, US

2019-01-01 to present | Chief Science Officer
Employment
Source: Self-asserted source
Thomas Epps, III

University of Delaware: Newark, DE, US

2006 to present | Allan & Myra Ferguson Distinguished Professor (Chemical and Biomolecular Engineering)
Employment
Source: Self-asserted source
Thomas Epps, III

NIST: Gaithersburg, MD, US

2004-08-01 to 2006-05-31 | NRC Postdoctoral Fellow (Polymers Division)
Employment
Source: Self-asserted source
Thomas Epps, III

Education and qualifications (1)

University of Minnesota: Minneapolis, MN, US

1999-09 to 2004-08 | Ph.D. (Chemical Engineering)
Education
Source: Self-asserted source
Thomas Epps, III

Works (50 of 153)

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Toward Sustainable Materials: From Lignocellulosic Biomass to High-Performance Polymers

Accounts of Materials Research
2025-02-21 | Journal article
Contributors: Jignesh S. Mahajan; Eric R. Gottlieb; Jung Min Kim; Thomas H. Epps, III
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Increased hydrophilicity of lignin-derivable vs. bisphenol-based polysulfones for potential water filtration applications

RSC Sustainability
2024 | Journal article
Contributors: Jignesh S. Mahajan; Hoda Shokrollahzadeh Behbahani; Matthew D. Green; LaShanda T. J. Korley; Thomas H. Epps
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Crossref

Lignin-derivable, thermoplastic, non-isocyanate polyurethanes with increased hydrogen-bonding content and toughness vs. petroleum-derived analogues

Materials Advances
2024 | Journal article
Contributors: Jignesh S. Mahajan; Zachary R. Hinton; Eduardo Nombera Bueno; Thomas H. Epps, III; LaShanda T. J. Korley
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Crossref

Cross-Linked Polyolefins: Opportunities for Fostering Circularity Throughout the Materials Lifecycle

ACS Applied Polymer Materials
2024-10-11 | Journal article
Contributors: Alison J. Shapiro; Paul J. Brigandi; Maria Moubarak; Saurav S. Sengupta; Thomas H. Epps, III
Source: check_circle
Crossref

Analyses of circular solutions for advanced plastics waste recycling

Nature Chemical Engineering
2024-10-10 | Journal article
Contributors: Kevin D. Nixon; Zoé O. G. Schyns; Yuqing Luo; Marianthi G. Ierapetritou; Dionisios G. Vlachos; LaShanda T. J. Korley; Thomas H. Epps, III
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Crossref

Tracking Chain Populations and Branching Structure during Polyethylene Deconstruction Processes

ACS Central Science
2024-09-25 | Journal article
Contributors: Alex H. Balzer; Zachary R. Hinton; Brandon C. Vance; Dionisios G. Vlachos; LaShanda T. J. Korley; Thomas H. Epps, III
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Crossref

Catalytic Deconstruction of Ethylene Vinyl Acetate Copolymer and Polyethylene Mixtures via Hydroconversion: Challenges and Solutions

ACS Sustainable Chemistry & Engineering
2024-06-10 | Journal article
Contributors: Pedro Moura; Pavel A. Kots; Brandon C. Vance; Zoé O. G. Schyns; Sean Najmi; Zachary R. Hinton; Caitlin M. Quinn; Thomas H. Epps, III; LaShanda T.J. Korley; Dionisios G. Vlachos
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Crossref

Toward Circular Recycling of Polyurethanes: Depolymerization and Recovery of Isocyanates

JACS Au
2024-04-22 | Journal article
Contributors: Robert M. O’Dea; Mridula Nandi; Genevieve Kroll; Jackie R. Arnold; LaShanda T. J. Korley; Thomas H. Epps, III
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Crossref

Which Lipid Nanoparticle (LNP) Designs Work? A Simple Kinetic Model Linking LNP Chemical Structure to In Vivo Delivery Performance

ACS Applied Materials & Interfaces
2024-03-20 | Journal article
Contributors: Esther H. Roh; Millicent O. Sullivan; Thomas H. Epps, III
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Crossref

Size and Structure Effects of Carbon-Supported Ruthenium Nanoparticles on Waste Polypropylene Hydrogenolysis Activity, Selectivity, and Product Microstructure

ACS Catalysis
2024-03-01 | Journal article
Contributors: Jessie A. Sun; Pavel A. Kots; Zachary R. Hinton; Nebojsa S. Marinkovic; Lu Ma; Steven N. Ehrlich; Weiqing Zheng; Thomas H. Epps, III; LaShanda T.J. Korley; Dionisios G. Vlachos
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Crossref

Solid-State, Single-Ion Conducting, Polymer Blend Electrolytes with Enhanced Li+ Conduction, Electrochemical Stability, and Limiting Current Density

Chemistry of Materials
2024-02-27 | Journal article
Contributors: Mengying Yang; Thomas H. Epps, III
Source: check_circle
Crossref

Electrophoretic Deposition as a Versatile Low-Cost Tool to Construct a Synthetic Polymeric Solid-Electrolyte Interphase on Silicon Anodes: A Model System Investigation

ACS Applied Materials & Interfaces
2024-02-14 | Journal article
Contributors: Rownak J. Mou; Sattajit Barua; Ajay K. Prasad; Thomas H. Epps, III; Koffi P. C. Yao
Source: check_circle
Crossref

Increase in the effective viscosity of polyethylene under extreme nanoconfinement

The Journal of Chemical Physics
2024-01-14 | Journal article
Contributors: Tian Ren; Zachary R. Hinton; Renjing Huang; Thomas H. Epps, III; LaShanda Korley; Raymond J. Gorte; Daeyeon Lee
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Crossref

Circularity in polymers: addressing performance and sustainability challenges using dynamic covalent chemistries

Chemical Science
2023 | Journal article
Contributors: Tianwei Yan; Alex H. Balzer; Katie M. Herbert; Thomas H. Epps; LaShanda T. J. Korley
Source: check_circle
Crossref

Lignin-derivable alternatives to petroleum-derived non-isocyanate polyurethane thermosets with enhanced toughness

Materials Advances
2023 | Journal article
Contributors: Sampanna V. Mhatre; Jignesh S. Mahajan; Thomas H. Epps; LaShanda T. J. Korley
Source: check_circle
Crossref

Unlocking Circularity Through the Chemical Recycling and Upcycling of Lignin-Derivable Polymethacrylates

Macromolecules
2023-12-12 | Journal article
Contributors: Ty Christoff-Tempesta; Robert M. O’Dea; Thomas H. Epps, III
Source: check_circle
Crossref

Thermogravimetric Analysis as a High-Throughput Lignocellulosic Biomass Characterization Method

ACS Sustainable Chemistry & Engineering
2023-12-11 | Journal article
Contributors: Alison J. Shapiro; Robert M. O’Dea; Thomas H. Epps, III
Source: check_circle
Crossref

Role of Intra-Domain Heterogeneity on Ion and Polymer Dynamics in Block Polymer Electrolytes: An Approach for Spatially Resolving Dynamics and Ion Transport

Macromolecules
2023-11-14 | Journal article
Contributors: Priyanka M. Ketkar; Nicholas F. Pietra; Andrew G. Korovich; Louis A. Madsen; Thomas H. Epps, III
Source: check_circle
Crossref

Role of Intradomain Heterogeneity on Ion and Polymer Dynamics in Block Polymer Electrolytes: Investigating Interfacial Mobility and Ion-Specific Dynamics and Transport

Macromolecules
2023-11-14 | Journal article
Contributors: Nicholas F. Pietra; Andrew G. Korovich; Priyanka M. Ketkar; Thomas H. Epps, III; Louis A. Madsen
Source: check_circle
Crossref

Ionic-Liquid-Mediated Deconstruction of Polymers for Advanced Recycling and Upcycling

ACS Macro Letters
2023-08-15 | Journal article
Contributors: Ty Christoff-Tempesta; Thomas H. Epps, III
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Crossref

Engineering Innovations, Challenges, and Opportunities for Lignocellulosic Biorefineries: Leveraging Biobased Polymer Production

Annual Review of Chemical and Biomolecular Engineering
2023-06-07 | Journal article
Part of ISSN: 1947-5438
Part of ISSN: 1947-5446
Contributors: Alison J. Shapiro; Robert M. O'Dea; Sonia C. Li; Jamael C. Ajah; Garrett F. Bass; Thomas H. Epps,
Source: Self-asserted source
Thomas Epps, III

Monitoring the Solution Persistence of Porous Coordination Cages with Diffusion NMR Spectroscopy and Cryogenic Transmission Electron Microscopy

The Journal of Physical Chemistry C
2023-02-09 | Journal article
Contributors: Garrett A. Taggart; Aynur Guliyeva; Kyunghee Kim; Glenn P. A. Yap; Darrin J. Pochan; Thomas H. Epps, III; Eric D. Bloch
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Crossref

Vat 3D Printing of Bioderivable Photoresins – Toward Sustainable and Robust Thermoplastic Parts

ACS Sustainable Chemistry & Engineering
2023-02-06 | Journal article
Contributors: Kyle C. H. Chin; Jianxun Cui; Robert M. O’Dea; Thomas H. Epps, III; Andrew J. Boydston
Source: check_circle
Crossref

Antioxidant-induced transformations of a metal-acid hydrocracking catalyst in the deconstruction of polyethylene waste

Green Chemistry
2022 | Journal article
Contributors: Zachary R. Hinton; Pavel A. Kots; Mya Soukaseum; Brandon C. Vance; Dionisios G. Vlachos; Thomas H. Epps; LaShanda T. J. Korley
Source: check_circle
Crossref

A kinetic modeling platform for predicting the efficacy of siRNA formulations in vitro and in vivo

STAR Protocols
2022-12 | Journal article
Contributors: Esther H. Roh; Millicent O. Sullivan; Thomas H. Epps, III
Source: check_circle
Crossref

Oxidative Functionalization of Long-Chain Liquid Alkanes by Pulsed Plasma Discharges at Atmospheric Pressure

ACS Sustainable Chemistry & Engineering
2022-12-05 | Journal article
Contributors: Darien K. Nguyen; Panagiotis Dimitrakellis; Michael R. Talley; Robert M. O’Dea; Thomas H. Epps, III; Mary P. Watson; Dionisios G. Vlachos
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Crossref

A Life Cycle Greenhouse Gas Model of a Yellow Poplar Forest Residue Reductive Catalytic Fractionation Biorefinery

Environmental Engineering Science
2022-10-01 | Journal article
Contributors: Yuqing Luo; Robert M. O'Dea; Yagya Gupta; Jeffrey Chang; Sunitha Sadula; Li Pei Soh; Allison M. Robbins; Delphis F. Levia; Dionisios G. Vlachos; Thomas H. Epps, III et al.
Source: check_circle
Crossref

Innovations Toward the Valorization of Plastics Waste

Annual Review of Materials Research
2022-07-01 | Journal article
Part of ISSN: 1531-7331
Part of ISSN: 1545-4118
Contributors: Zachary R. Hinton; Michael R. Talley; Pavel A. Kots; Anne V. Le; Tan Zhang; Michael E. Mackay; Aditya M. Kunjapur; Peng Bai; Dionisios G. Vlachos; Mary P. Watson et al.
Source: Self-asserted source
Thomas Epps, III

A kinetic modeling platform for predicting the efficacy of siRNA formulations in vitro and in vivo

2022-06-06 | Preprint
Contributors: Esther H Roh; Millicent O. Sullivan; Thomas H. Epps, III
Source: check_circle
Crossref

Sustainability of Synthetic Plastics: Considerations in Materials Life-Cycle Management

JACS Au
2022-01-24 | Journal article
Contributors: Thomas H. Epps, III; LaShanda T. J. Korley; Tianwei Yan; Kathryn L. Beers; Tiffani M. Burt
Source: check_circle
Crossref

Ambient-pressure lignin valorization to high-performance polymers by intensified reductive catalytic deconstruction

Science Advances
2022-01-21 | Journal article | Author
Part of ISSN: 2375-2548
Contributors: Robert O'Dea; Paula A. Pranda; Yuqing Luo; Alice Amitrano; Elvis Osamudiamhen Ebikade; Eric Gottlieb; Olumoye A. Ajao; Marzouk Benali; Dionisios Vlachos; Marianthi Ierapetritou et al.
Source: Self-asserted source
Thomas Epps, III

Inline Rolling Shear Alignment: Deposition and Long-Range Order of Block Polymer Templates in a Fast, Single-Step Process

ACS Applied Polymer Materials
2022-01-14 | Journal article
Contributors: Eric R. Gottlieb; Panagiotis Dimitrakellis; Dionisios G. Vlachos; Thomas H. Epps, III
Source: check_circle
Crossref

Estrogenic activity of lignin-derivable alternatives to bisphenol A assessed via molecular docking simulations

RSC Advances
2021 | Journal article
Contributors: Alice Amitrano; Jignesh S. Mahajan; LaShanda T. J. Korley; Thomas H. Epps
Source: check_circle
Crossref

Recent developments towards performance-enhancing lignin-based polymers

Polymer Chemistry
2021 | Journal article
Contributors: Garrett F. Bass; Thomas H. Epps
Source: check_circle
Crossref

Single pot catalyst strategy to branched products via adhesive isomerization and hydrocracking of polyethylene over platinum tungstated zirconia

Applied Catalysis B: Environmental
2021-12 | Journal article
Contributors: Brandon C. Vance; Pavel A. Kots; Cong Wang; Zachary R. Hinton; Caitlin M. Quinn; Thomas H. Epps, III; LaShanda T.J. Korley; Dionisios G. Vlachos
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Nanostructured Block Polymer Electrolytes: Tailoring Self-Assembly to Unlock the Potential in Lithium-Ion Batteries

Accounts of Chemical Research
2021-12-07 | Journal article
Contributors: Priyanka M. Ketkar; Thomas H. Epps, III
Source: check_circle
Crossref

Kinetic Modeling to Accelerate the Development of Nucleic Acid Formulations

ACS Nano
2021-10-26 | Journal article
Contributors: Esther H. Roh; Thomas H. Epps, III; Millicent O. Sullivan
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Crossref

From Lab to Fab: Enabling Enhanced Control of Block Polymer Thin-Film Nanostructures

ACS Applied Polymer Materials
2021-09-10 | Journal article
Contributors: Eric R. Gottlieb; Aynur Guliyeva; Thomas H. Epps, III
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Crossref

Quantifying the Effects of Monomer Segment Distributions on Ion Transport in Tapered Block Polymer Electrolytes

Macromolecules
2021-08-24 | Journal article
Contributors: Priyanka M. Ketkar; Kuan-Hsuan Shen; Mengdi Fan; Lisa M. Hall; Thomas H. Epps, III
Source: check_circle
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Entrepreneurship in Polymer Chemistry

ACS Macro Letters
2021-07-20 | Journal article
Contributors: Katrina M. Knauer; Joshua C. Speros; Lisa K. Kemp; Daniel A. Savin; Zhenan Bao; Geoffrey W. Coates; Thomas H. Epps, III; Craig J. Hawker; Jennifer J. Le Roy; Molly Morse et al.
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Toward polymer upcycling—adding value and tackling circularity

Science
2021-07-02 | Journal article
Contributors: LaShanda T. J. Korley; Thomas H. Epps, III; Brett A. Helms; Anthony J. Ryan
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Metal–organic framework polymer composite enhancement via acyl chloride modification

Polymer International
2021-06 | Journal article
Contributors: Gregory W Peterson; Hui Wang; Kathleen Au; Thomas H Epps, III
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Fibre-based composites from the integration of metal–organic frameworks and polymers

Nature Reviews Materials
2021-03-24 | Journal article
Contributors: Gregory W. Peterson; Dennis T. Lee; Heather F. Barton; Thomas H. Epps, III; Gregory N. Parsons
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Crossref

Redox Flow Battery Membranes: Improving Battery Performance by Leveraging Structure–Property Relationships

ACS Energy Letters
2021-01-08 | Journal article
Contributors: Craig A. Machado; Gerald O. Brown; Ruidong Yang; Timothy E. Hopkins; Julia G. Pribyl; Thomas H. Epps, III
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Bent‐But‐Not‐Broken: Reactive Metal‐Organic Framework Composites from Elastomeric Phase‐Inverted Polymers

Advanced Functional Materials
2020-12 | Journal article
Contributors: Gregory W. Peterson; John J. Mahle; Trenton M. Tovar; Thomas H. Epps, III
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Crossref

Aromatics from Lignocellulosic Biomass: A Platform for High-Performance Thermosets

ACS Sustainable Chemistry & Engineering
2020-10-12 | Journal article
Contributors: Jignesh S. Mahajan; Robert M. O’Dea; Joanne B. Norris; LaShanda T. J. Korley; Thomas H. Epps, III
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100th Anniversary of Macromolecular Science Viewpoint: Polymers from Lignocellulosic Biomass. Current Challenges and Future Opportunities

ACS Macro Letters
2020-04-21 | Journal article
Contributors: Robert M. O’Dea; Jordan A. Willie; Thomas H. Epps, III
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Dual‐functional, aromatic, epoxy‐methacrylate monomers from bio‐based feedstocks and their respective epoxy‐functional thermoplastics

Journal of Polymer Science
2020-03 | Journal article
Contributors: Alexander W. Bassett; Kayla R. Sweet; Robert M. O'Dea; Amy E. Honnig; Claire M. Breyta; Julia H. Reilly; John J. La Scala; Thomas H. Epps, III; Joseph F. Stanzione, III
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Block Copolymer Vitrimers

Journal of the American Chemical Society
2020-01-08 | Journal article
Contributors: Jacob J. Lessard; Georg M. Scheutz; Seung Hyun Sung; Kayla A. Lantz; Thomas H. Epps, III; Brent S. Sumerlin
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Charging toward improved lithium-ion polymer electrolytes: exploiting synergistic experimental and computational approaches to facilitate materials design

Molecular Systems Design & Engineering
2019 | Journal article
Contributors: Priyanka M. Ketkar; Kuan-Hsuan Shen; Lisa M. Hall; Thomas H. Epps
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Peer review (62 reviews for 12 publications/grants)

Review activity for ACS applied materials & interfaces. (5)
Review activity for ACS applied polymer materials. (7)
Review activity for ACS central science. (1)
Review activity for ACS energy letters. (3)
Review activity for ACS macro letters. (8)
Review activity for ACS nano. (1)
Review activity for ACS sustainable chemistry & engineering. (15)
Review activity for Advanced materials. (1)
Review activity for Biomacromolecules. (2)
Review activity for Chemistry of materials. (1)
Review activity for Journal of the American Chemical Society. (1)
Review activity for Macromolecules. (17)